Studying the Breit effects in actinides.
1) Petrov A.N., Mosyagin N.S., Titov A.V. 2) Tupitsyn I.I.
1) Petersburg Nuclear Physics Institute 2) St.-Petersburg State
University
In the present work we report the investigation of the low frequency
Breit effects for actinides. For this purpose, the finite-difference (numerical)
codes developed earlier for the Dirac-Hartree-Fock calculations with the
Breit interaction (DHFB) taken into account are applied. The contributions
of both instantaneous magnetic (Gaunt) and retardation of the Coulomb interaction
between electrons as well as contributions from/between
different shells are studied. The calculation of the Breit corrections
to the valence and core properties for the uranium, plutonium and other
atoms is performed. The quality of different relativistic effective core
potentials
(RECPs) is studied with respect to the DHFB calculations.
The work of A.P., N.M. and A.T. was supported by RFBR (grant N 03-03-32335).
A.P. is grateful to the Ministry of Education of the Russian Federation
ant
to St.-Petersburg Committee on Science and Higher Education for
the
Grant N PD02-1.3-236. A.T. and N.M. were supported in part by
Scientific Program of St.Petersburg Scientific Center of RAS.